Anything and everything Inu-Yasha. For such a badass Anime that actually turned into an repetitively bad Anime after the first 50 eps--there wasn't a single opening or ending that wasn't great. They are all memorable; I couldn't possibly list a single opening or ending and actually be sure about it. So I'll go with two different Anime's on the matter.
Best Opening -- Dan Dan Kokoro Hikareteku -- Dragon Ball GT
Best Ending -- Ryuusei -- Naruto
Last Exile - Cloud Age Symphony
Tenjou Tenge- Bomb a Head
Hellsing - A World Without Logos
Hunter x Hunter - Taiyou wa Yoru mo Kaga-yaku
Shin Seiki Evangelion - Cruel Angel's Thesis
Endings:
Yakitate!! Japan - Tor All Tha Dreamers
Naruto - Ryuusei
Hunter x Hunter - Pray
One Piece - Watashi ga Iru yo
One Piece - Shouchi no Suke
One Piece - Shining Ray
One Piece - Glory
Fate/Stay Night - Kirameku Namida wa Hoshi ni
Chobits - Ningyo Hime
I apologize for not elaborating properly. Which anime do you think has the best opening movie (before the episode starts) and/or best closing movie (after the episode is over).
I still think best OP/ED is in Elfen lied, the sadness of the music just fits in the series better than anything.
Otherwise FullMetal Alchemist has some of the best OP/EDs around
Best openings:
Lilium - Elfen lied OST
Rewrite - Asian kung fu generation - FMA
Best endings:
"Be your girl" - Elfen lied OST
Kesenai Tsumi - Nana Kitade - FMA
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